ΠροτεινόμεναΘέματακαιΑνάθεσηΔιπλωματικώνΕργασιών
Microwave-Assisted Continuous-Flow Synthesis of Carbonated Soybean Oil
under Pressurized Conditions
The global polyurethane (PU)
industry faces significant sustainability and safety challenges due to its
reliance on isocyanates, which are traditionally synthesized using highly toxic
phosgene and petroleum-based feedstocks. In response to these concerns,
Non-Isocyanate Polyurethanes (NIPUs) have emerged as a promising, eco-friendly
alternative. Carbonated Soybean Oil (CSBO) represents a renewable precursor for
the synthesis of NIPUs, produced via the cycloaddition of CO2 to
Epoxidized Soybean Oil (ESBO). While this gas-liquid reaction has traditionally
been limited to batch systems, this diploma thesis focuses on the design and
operation of a microwave-assisted continuous-flow tubular reactor for CSBO
production. The study experimentally investigates the homogeneous catalytic
reaction between CO2 and ESBO, aiming to identify optimal operating
parameters (pressure, temperature, and reactant flow rates) that maximize mass
transfer efficiency and reaction kinetics. Product quality is assessed via
epoxide conversion using a titration-based analytical method, FTIR and NMR
spectroscopy. Furthermore, the process is simulated using COMSOL Multiphysics
to model the temperature distribution and fluid dynamics along the reactor
length, providing a comprehensive understanding of the transport phenomena
governing the reactor's performance and scalability.
Επιβλέπων μέλος ΔΕΠ:
Γεώργιος Στεφανίδης
Τομέας: Ανάλυσης, Σχεδιασμού και Ανάπτυξης Διεργασιών και Συστημάτων
Σχετικό Μάθημα : Μηχανική Χημικών Διεργασιών ΙΙ
Περίοδος Ανάθεσης: Φεβρουαρίου Ακ. Έτους 2025-2026
Τομέας: Ανάλυσης, Σχεδιασμού και Ανάπτυξης Διεργασιών και Συστημάτων
Σχετικό Μάθημα : Μηχανική Χημικών Διεργασιών ΙΙ
Περίοδος Ανάθεσης: Φεβρουαρίου Ακ. Έτους 2025-2026





